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may refer to:
- Holy Roman Emperor Charles V, who was also known as Carlos I of Spain
- Don Carlos, Prince of Asturias, eldest son of Philip II of Spain
- Carlos, Infante of Spain, second surviving son of Philip III of Spain
- Baltasar Carlos, Prince of Asturias, eldest son of Philip IV of Spain
- Charles II of Spain - etc all kings Charles of Spain
- Infante Carlos of Spain, Count of Molina, pretender as Carlos V (the first claimant king of Spanish Carlism) and the second surviving son of Charles IV of Spain
- Carlos, Count of Montemolin, Carlist pretender as Carlos VI
- Carlos, Duke of Madrid, Carlist pretender as Carlos VII
- Alfonso Carlos, Duke of San Jaime, Carlist pretender
- Archduke Karl Pius, Prince of Tuscany, leader of breakaway Carlist movement between 1943 and 1953 and a disputed pretender as Carlos VIII
- Carlos Hugo, Duke of Parma, former Carlist Prince of Asturias
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